Circular dichroism is a consequence of chirality. However, nonchiral molecules can also exhibit it when the measurement itself introduces chirality, e.g., when measuring molecular-frame photoelectron angular distributions. The few such... more
Photoelectron angular distributions from fixed-in-space H 2 molecules exposed to ultrashort xuv laser pulses have been evaluated. The theoretical method is based on the solution of the time-dependent Schrödinger equation in a basis of... more
The authors present evidence for a distinct optical phonon progression in the nonlinear intersubband absorption spectra of electrons in a GaN∕AlN superlattice. Femtosecond two-color pump-probe experiments in the near infrared show... more
Near single-cycle terahertz pulse generation from lithium niobate crystal by optical rectification of pulses from an Yb:fiber laser/amplifier system was investigated. The pump laser supplied 250 fs duration pulses with 14 μJ energy at up... more
Submitted for the MAR10 Meeting of The American Physical Society Molecular dynamics simulations of ablation and spallation of gold irradiated by femtosecond laser
The ability of pellets made up of compressed iron iodate nanocrystals to frequency-double the whole visible spectrum is demonstrated. We suggest their use for complete characterization of intense ultrabroadband laser pulses.
We demonstrate that a driving ultrashort laser pulse undergoing filamentation can induce a remarkably large birefringence in Argon, resulting in an ultrafast "half-wave plate" for a copropagating non-filamenting probe beam. Such... more
We propose the impingement of non-uniform wavefront curvature as a simple way to improve the longitudinal homogeneity of the plasma density along filaments generated by ultrashort laser pulses. We characterize multiple filamentation of a... more
Stark spectroscopy, which is well established for probing transitions between the ground and excited states of many material classes, is extended to transitions between transient excited states. To this end, it is combined with... more
In conjugated polymers excited singlet states are known to dissociate into polarons upon application of an electric field. We show that for excitation intensities exceeding 100 J cm -2 in polyfluorene, this is not the only mechanism of... more
We studied the hyperfine structure and hyperfine coherent properties of the 3 H 4 ͑0͒ → 1 D 2 ͑0͒ transition of Pr 3+ ions in a tungstate single crystal La 2 ͑WO 4 ͒ 3 by hole-burning and photon-echo techniques. This work is motivated by... more
Decreasing the pulse duration helps confine damage, shorten treatment time, and minimize pain during retinal photocoagulation. However, the safe therapeutic window (TW), the ratio of threshold powers for thermomechanical rupture of... more
We demonstrate submicron resolution imaging using picosecond acoustic phonon pulses. High-frequency acoustic pulses are generated by impulsive thermoelastic excitation of a patterned 15-nm-thick metal film on a crystalline substrate using... more
We study the feasibility of femtosecond laser writing of optical waveguides in bulk 35PbO∙35Bi2O3∙15Ga2O3∙15GeO2 glass, motivated by the extended transparency interval of heavy metal oxide glasses in the mid-infrared regime. Its large... more
A laser based electron generator is shown, for the first time, to produce sufficient charge to conduct time resolved investigations of radiation induced chemical events. Electron pulses generated by focussing terawatt laser pulses into a... more
We report the fabrication of waveguides in lithium tantalate using a 250 kHz high-repetition rate ultrafast laser at 771 nm and the characterization of the resulting laser induced structure with second harmonic microscopy. Waveguides... more
To produce accurate data from optical streak cameras requires accurate temporal calibration sources. We have reproduced an older technology for generating optical timing marks that had been lost due to component availability. Many... more
Accumulation of thermal energies by highly repeated irradiation of femtosecond laser pulses inside a glass induces the heat-modification whose volume is much larger than that of the photoexcited region. It has been proposed that the... more
Accumulation of thermal energies by highly repeated irradiation of femtosecond laser pulses inside a glass induces the heat-modification whose volume is much larger than that of the photoexcited region. It has been proposed that the... more
Photon-induced ultrafast energy dissipation in small isolated Ni 3 Ϫ has been studied by two-color pumpprobe photoelectron spectroscopy. The time-resolved photoelectron spectra clearly trace the path from a singleelectron excitation to a... more
Nonlinear optical media that are normally dispersive, support a new type of localized (nondiffractive and nondispersive) wavepackets that are X-shaped in space and time and have slower than exponential decay. High-intensity X-waves,... more
We study the generation of subfemtosecond pulses with the molecular coherence control in stimulated Raman scattering. We show analytically that the antiphased state temporally advances the higher frequencies with respect to the lower... more
Terahertz microcavity lasers with subwavelength mode volumes and thresholds in the milliampere range
The authors demonstrate terahertz microcavity lasers with ultralow current thresholds ͑I th Ϸ 4 mA͒ and with reduced mode volumes of Ϸ0.7͑ effective ͒ 3 , i.e., less than one cubic wavelength. A double metal waveguide with reduced active... more
Mode locking based on an epitaxial composite of the monoclinic double tungstate crystal Yb: KLu͑WO 4 ͒ 2 is realized. A 100 m thin Yb: KLu͑WO 4 ͒ 2 layer grown on a KLu͑WO 4 ͒ 2 substrate is used as an active medium in a laser passively... more
We demonstrate an all-optical circuit capable of generating 40-GHz control signals from f lag pulses that can be used to define the switching state of all-optical gates for use with optical packets. The circuit comprises a Fabry-Perot... more
We have built a diode-pumped Nd : glass regenerative amplifier that is able to produce energies up to 20 mJ within a 470-fs pulse duration at a 1-Hz repetition rate. We obtained this amplifier by using specific intracavity components such... more
Optical pulses of 200 fs with 165 W of peak power have been generated from an AlGaAs semiconductor diodelaser system. These pulses represent, to our knowledge, both the shortest and most intense ever generated from an all-semiconductor... more
Circular dichroism is a consequence of chirality. However, nonchiral molecules can also exhibit it when the measurement itself introduces chirality, e.g., when measuring molecular-frame photoelectron angular distributions. The few such... more
Photoelectron angular distributions from fixed-in-space H 2 molecules exposed to ultrashort xuv laser pulses have been evaluated. The theoretical method is based on the solution of the time-dependent Schrödinger equation in a basis of... more
The dynamics of nonlinear optical conversion in the high-intensity femtosecond pump regime has been studied in gaseous media over a wide pressure range. The existence of two different types of optical supercontinua, structured and... more
What we believe is a new scheme for producing semidiscrete self-trapped vortices ("swirling photon droplets") in photonic crystals with competing quadratic (χ (2)) and selfdefocusing cubic (χ (3)) nonlinearities is proposed. The photonic... more
Public reporting burden for this collection of information is estimated to average 1 hour per response, including the time for reviewing instructions, searching existing data sources, gathering and maintaining the data needed, and... more
Ultrafast thin disk laser oscillators achieve the highest average output powers and pulse energies of any mode-locked laser oscillator technology. The thin disk concept avoids thermal problems occurring in conventional high-power rod or... more
We describe recent results and developments in the preamplifier module (PAM) engineering prototype located in NIF's front end or Optical Pulse Generation (OPG) system. This prototype uses the general laser design developed on a physics... more
Terahertz (THz) radiation has been observed from multiferroic BiFeO3 thin films via ultrafast modulation of spontaneous polarization upon carrier excitation with illumination of femtosecond laser pulses. The radiated THz pulses from... more
Generation and characterization of spatially and temporally localized few-cycle optical wave packets
Direct experimental evidence of localized few-cycle wave packets with a characteristic spatiotemporal X shape is reported. These wave packets are also referred to as X pulses. For their generation, a Ti:sapphire laser beam was transformed... more
We report the experimental observation and the theoretical modeling of self-induced-transparency signatures such as nonlinear transmission, pulse retardation and reshaping, for subpicosecond pulse propagation in a 2-mm-long InGaAs... more
We compare the performance of two quantum dot saturable absorber mirrors with one device operating at the quantum dot ground state transition whereas the other operates at the first excited state transition. Time-resolved... more
We describe a novel electro-optic double-modulation (DM) sampling technique for ultrafast transient spectroscopy, which is characterized by a superior signal-to-noise ratio compared to that of a regular single-modulation technique. DM is... more
The nonlinear polarization close to the band gap of GaAs is studied by spectrally and temporally resolved four-wave mixing. Excitonic and free carrier contributions both excited within the bandwidth of the 100 fs pulses are distinguished... more
We study the generation of a self-chirped optical pulse in a free-electron laser (FEL) oscillator. In a high-gain FEL oscillator, the frequency chirp is induced in the slippage region as a result of superradiant FEL resonance, and this... more
It is demonstrated in a numerical simulation that an intense fs keV x-ray pulse can be generated by the interaction of a tightly focused femtosecond laser copropagating with an electron bunch. In general, the interaction of a loosely... more
We report a fiber-based, pulsed laser seeder system that rapidly switches among 6 wavelengths across atmospheric carbon dioxide (CO 2) absorption line near 1572.3 nm for measurements of global CO 2 mixing ratios to 1-ppmv precisiqn. One... more
A fast-scan method was developed to obtain time-resolved signals with femtosecond resolution over a picosecond range on the fly and in real time. Traditional fast-scan methods collect data at each probe wavelength one by one, which is... more
A high-resolution second-harmonic optical coherence tomography (SH-OCT) system is demonstrated using a spectrum broadened femtosecond Ti:sapphire laser. An axial resolution of 4.2μm at the second-harmonic wave center wavelength of 400 nm... more
The effects of dispersion on the pulsewidth of a mode-locked fiber ring laser are examined. We have identified two different modes of operation, one where the pulsewidth is determined by the path-integrated (global) dispersion of the... more