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2006, Nature
Competition between electronic ground states near a quantum critical point (QCP) - the location of a zero-temperature phase transition driven solely by quantum-mechanical fluctuations - is expected to lead to unconventional behaviour in low-dimensional systems. New electronic phases of matter have been predicted to occur in the vicinity of a QCP by two-dimensional theories, and explanations based on these ideas have been proposed for significant unsolved problems in condensed-matter physics, such as non-Fermi-liquid behaviour and high-temperature superconductivity. But the real materials to which these ideas have been applied are usually rendered three-dimensional by a finite electronic coupling between their component layers; a two-dimensional QCP has not been experimentally observed in any bulk three-dimensional system, and mechanisms for dimensional reduction have remained the subject of theoretical conjecture. Here we show evidence that the Bose-Einstein condensate of spin triplets in the three-dimensional Mott insulator BaCuSi2O6 provides an experimentally verifiable example of dimensional reduction at a QCP. The interplay of correlations on a geometrically frustrated lattice causes the individual two-dimensional layers of spin-1/2 Cu2+ pairs (spin dimers) to become decoupled at the QCP, giving rise to a two-dimensional QCP characterized by power law scaling distinctly different from that of its three-dimensional counterpart. Thus the very notion of dimensionality can be said to acquire an 'emergent' nature: although the individual particles move on a three-dimensional lattice, their collective behaviour occurs in lower-dimensional space.
Science, 2000
Published in Science 288, 475 (2000).
Physical Review B, 2013
In order to understand the nature of the two-dimensional Bose-Einstein condensed (BEC) phase in BaCuSi2O6, we performed detailed 63 Cu and 29 Si NMR above the critical magnetic field, Hc1 = 23.4 T. The two different alternating layers present in the system have very different local magnetizations close to Hc1; one is very weak, and its size and field dependence are highly sensitive to the nature of inter-layer coupling. Its precise value could only be determined by "onsite" 63 Cu NMR, and the data are fully reproduced by a model of interacting hard-core bosons in which the perfect frustration associated to tetragonal symmetry is slightly lifted, leading to the conclusion that the population of the less populated layers is not fully incoherent but must be partially condensed.
Physical Review Letters, 2007
We show that the spatial dimensionality of the quantum critical point associated with Bose-Einstein condensation at T 0 is reduced when the underlying lattice comprises layers coupled by a frustrating interaction. Our theoretical predictions for the critical behavior correspond very well with recent measurements in
1999
For intermediate Coulomb energy to Fermi energy ratios rs, spinless fermions in a random potential form a new quantum phase which is different from the Fermi glass and the Wigner crystal. From a numerical study of small clusters, we show that this phase is characterized by an ordered flow of enhanced persistent currents and occurs for rs values where a metallic phase has been observed in two dimensions.
Physical Review B, 2020
We explore several classes of quadrupolar ordering in a system of antiferromagnetically coupled quantum spin-1 dimers, which are stacked in the triangular lattice geometry forming a bilayer. Lowenergy properties of this model is described by an S = 1 hard-core bosonic degrees of freedom defined on each dimer-bond, where the singlet and triplet states of the dimerized spins are interpreted as the vacuum and the occupancy of boson, respectively. The number of bosons per dimer and the magnetic and density fluctuations of bosons are controlled by the inter-dimer Heisenberg interactions. In a solid phase where each dimer hosts one boson and the inter-dimer interaction is weak, a conventional spin nematic phase is realized by the pair-fluctuation of bosons. Larger inter-dimer interaction favors Bose Einstein condensates (BEC) carrying quadrupolar moments. Among them, we find one exotic phase where the quadrupoles develop a spatially modulated structure on the top of a uniform BEC, interpreted in the original dimerized spin-1 model as coexistent p-type nematic and 120 • -magnetic correlations. This may explain an intriguing nonmagnetic phase found in Ba3ZnRu2O9.
Physical Review B, 2004
We present the critical theory of a number of zero temperature phase transitions of quantum antiferromagnets and interacting boson systems in two dimensions. The most important example is the transition of the S = 1/2 square lattice antiferromagnet between the Néel state (which breaks spin rotation invariance) and the paramagnetic valence bond solid (which preserves spin rotation invariance but breaks lattice symmetries). We show that these two states are separated by a secondorder quantum phase transition. This conflicts with Landau-Ginzburg-Wilson theory, which predicts that such states with distinct broken symmetries are generically separated either by a first-order transition, or by a phase with co-existing orders. The critical theory of the second-order transition is not expressed in terms of the order parameters characterizing either state, but involves fractionalized degrees of freedom and an emergent, topological, global conservation law. A closely related theory describes the superfluid-insulator transition of bosons at half-filling on a square lattice, in which the insulator has a bond density wave order. Similar considerations are shown to apply to transitions of antiferromagnets between the valence bond solid and the Z2 spin liquid: the critical theory has deconfined excitations interacting with an emergent U(1) gauge force. We comment on the broader implications of our results for the study of quantum criticality in correlated electron systems.
Physical Review Letters, 2012
The liquid and crystal phase of a single-component Fermi gas with dipolar interactions are investigated using quantum Monte Carlo methods in two spatial dimensions and at zero temperature. The dipoles are oriented by an external field perpendicular to the plane of motion, resulting in a purely repulsive 1/r 3 interaction. In the liquid phase we calculate the equation of state as a function of the interaction strength and other relevant properties characterizing the Fermi-liquid behavior: effective mass, discontinuity at the Fermi surface and pair correlation function. In the high density regime we calculate the equation of state of the Wigner crystal phase and the critical density of the liquid to solid first order phase transition. Close to the freezing density we also search for the existence of a stripe phase, but such a phase is never found to be energetically favorable. PACS numbers: 05.30.Fk, 03.75.Hh, 03.75.Ss
arXiv (Cornell University), 2015
Increasing the spin imbalance in superconductors can spatially modulate the gap by forming Cooper pairs with finite momentum. For large imbalances compared to the Fermi energy, the inhomogeneous FFLO superconductor ultimately becomes a normal metal. There is mounting experimental evidence for this scenario in 2D organic superconductors in large in-plane magnetic fields; this is complemented by ongoing efforts to realize this scenario in coupled tubes of atomic Fermi gases with spin imbalance. Yet, a theory for the phase transition from a metal to an FFLO superconductor has not been developed so far and the universality class has remained unknown. Here we propose and analyze a spin imbalance driven quantum critical point between a 2D metal and an FFLO phase in anisotropic electron systems. We derive the effective action for electrons and bosonic FFLO pairs at this quantum phase transition. Using this action, we predict non-Fermi liquid behavior and the absence of quasi-particles at a discrete set of hot spots on the Fermi surfaces. This results in strange power-laws in thermodynamics and response functions, which are testable with existing experimental setups on 2D organic superconductors and may also serve as signatures of the elusive FFLO phase itself. The proposed universality class is distinct from previously known quantum critical metals and, because its critical fluctuations appear already in the pairing channel, a promising candidate for naked metallic quantum criticality over extended temperature ranges.
To understand the complex physics of a system with strong electron-electron interactions, the ideal is to control and monitor its properties while tuning an external electric field applied to the system (the electric-field effect). Indeed, complete electricfield control of many-body states in strongly correlated electron systems is fundamental to the next generation of condensed matter research and devices 1-3 . However, the material must be thin enough to avoid shielding of the electric field in the bulk material. Twodimensional materials do not experience electrical screening, and their charge-carrier density can be controlled by gating. Octahedral titanium diselenide (1T-TiSe 2 ) is a prototypical twodimensional material that reveals a charge-density wave (CDW) and superconductivity in its phase diagram 4 , presenting several similarities with other layered systems such as copper oxides 5 , iron pnictides 6 , and crystals of rare-earth elements and actinide atoms 7 . By studying 1T-TiSe 2 single crystals with thicknesses of 10 nanometres or less, encapsulated in two-dimensional layers of hexagonal boron nitride, we achieve unprecedented control over the CDW transition temperature (tuned from 170 kelvin to 40 kelvin), and over the superconductivity transition temperature (tuned from a quantum critical point at 0 kelvin up to 3 kelvin). Electrically driving TiSe 2 over different ordered electronic phases allows us to study the details of the phase transitions between many-body states. Observations of periodic oscillations of magnetoresistance induced by the Little-Parks effect show that the appearance of superconductivity is directly correlated with the spatial texturing of the amplitude and phase of the superconductivity order parameter, corresponding to a two-dimensional matrix of superconductivity. We infer that this superconductivity matrix is supported by a matrix of incommensurate CDW states embedded in the commensurate CDW states. Our results show that spatially modulated electronic states are fundamental to the appearance of two-dimensional superconductivity.
Journal of Experimental and Theoretical Physics, 2000
The effect of static fluctuations in the phase of the order parameter on the normal and superconducting properties of a 2D system with attractive fourfermion interaction is studied. Analytic expressions for the fermion Green's function, its spectral density, and the density of states are derived in the approximation where the coupling between the spin and charge degrees of freedom is neglected. The resulting single-particle Green's function clearly demonstrates a non-Fermi liquid behavior. The results show that as the temperature increases through the 2D critical temperature, the width of the quasiparticle peaks broadens significantly.
Nature Materials, 2013
The diverse phenomena associated with the two-dimensional electron gas (2DEG) that occurs at oxide interfaces include, among others, exceptional carrier mobilities, magnetism and superconductivity. Although these have mostly been the focus of interest for potential future applications, they also offer an opportunity for studying more fundamental quantum many-body effects. Here, we examine the magnetic-field-driven quantum phase transition that occurs in electrostatically gated superconducting LaTiO 3 /SrTiO 3 interfaces. Through a finite-size scaling analysis, we show that it belongs to the (2 + 1)D XY model universality class. The system can be described as a disordered array of superconducting puddles coupled by a 2DEG and, depending on its conductance, the observed critical behaviour is single (corresponding to the long-range phase coherence in the whole array) or double (one related to local phase coherence, the other one to the array). A phase diagram illustrating the dependence of the critical field on the 2DEG conductance is constructed, and shown to agree with theoretical proposals. Moreover, by retrieving the coherence-length critical exponent ν, we show that the quantum critical behaviour can be clean or dirty according to the Harris criterion, depending on whether the phase-coherence length is smaller or larger than the size of the puddles.
Physical Review E, 2020
We revisit the problem of the reduction of the three-dimensional (3D) dynamics of Bose-Einstein condensates, under the action of strong confinement in one direction (z), to a 2D mean-field equation. We address this problem for the confining potential with a singular term, viz., V z (z) = 2z 2 + ζ 2 /z 2 , with constant ζ. A quantum phase transition is induced by the latter term, between the ground state (GS) of the harmonic oscillator and the 3D condensate split in two parallel non-interacting layers, which is a manifestation of the "superselection" effect. A realization of the respective physical setting is proposed, making use of resonant coupling to an optical field, with the resonance detuning modulated along z. The reduction of the full 3D Gross-Pitaevskii equation (GPE) to the 2D nonpolynomial Schrödinger equation (NPSE) is based on the factorized ansatz, with the z-dependent multiplier represented by an exact GS solution of the 1D Schrödinger equation with potential V(z). For both repulsive and attractive signs of the nonlinearity, the 2D NPSE produces GS and vortex states, that are virtually indistinguishable from the respective numerical solutions provided by full 3D GPE. In the case of the self-attraction, the threshold for the onset of the collapse, predicted by the 2D NPSE, is also virtually identical to its counterpart obtained from the 3D equation. In the same case, stability and instability of vortices with topological charge S = 1, 2, and 3 are considered in detail. Thus, the procedure of the spatial-dimension reduction, 3D → 2D, produces very accurate results, and it may be used in other settings.
Physical review letters, 2018
We study the temperature dependence of the electrical resistivity in a system composed of critical spin chains interacting with three-dimensional conduction electrons and driven to criticality via an external magnetic field. The relevant experimental system is Yb_{2}Pt_{2}Pb, a metal where itinerant electrons coexist with localized moments of Yb ions which can be described in terms of effective S=1/2 spins with a dominantly one-dimensional exchange interaction. The spin subsystem becomes critical in a relatively weak magnetic field, where it behaves like a Luttinger liquid. We theoretically examine a Kondo lattice with different effective space dimensionalities of the two interacting subsystems. We characterize the corresponding non-Fermi liquid behavior due to the spin criticality by calculating the electronic relaxation rate and the dc resistivity and establish its quasilinear temperature dependence.
The European Physical Journal B
Proximity to magnetic order as well as low dimensionality are both beneficial to superconductivity at elevated temperatures. Materials on the border of magnetism display a wide range of novel and potentially useful phenomena: high Tcs, heavy fermions, coexistence of magnetism and superconductivity and giant magnetoresistance. Low dimensionality is linked to enhanced fluctuations and, in the case of heavy fermions, has been experimentally shown to be beneficial for the fluctuations that are responsible for the rich abundance of novel emergent phases. This experimental strategy motivated us to explore 2D insulating magnets with a view to investigate phase evolution across metal-insulator and magnetic-non-magnetic boundaries. This has been a fruitful venture with totally novel results different to our expectations. We present results from 2 distinct systems. The MPS3 family are highly anisotropic in both their crystal and magnetic structures. FePS3 in particular is a model insulating honeycomb antiferromagnet. We find that the application of pressure to FePS3 induces an insulator to metal transition. The second system, Cs2CuCl4, is a highly-frustrated quantum spin liquid at low temperature. The competition of the 3 relevant exchange couplings is delicately balanced. It has been shown to become antiferromagnetic at very low temperatures (∼1 K). We have found that the application of pressure for 3 days or more followed by a return to ambient pressure stabilises a totally distinct magnetic ground state.
Physical Review B, 2007
We analyze the spin relaxation time 1/T1 for a system made of weakly coupled one dimensional ladders. This system allows to probe the dimensional crossover between a Luttinger liquid and a Bose-Einstein condensate of magnons. We obtain the temperature dependence of 1/T1 in the various dimensional regimes, and discuss the experimental consequences.
Physical Review B, 2011
In certain Mott-insulating dimerized antiferromagnets, triplet excitations of the paramagnetic phase can decay into the two-particle continuum. When such a magnet undergoes a quantum phase transition into a magnetically ordered state, this coupling becomes part of the critical theory provided that the lattice ordering wavevector is zero. One microscopic example is the staggered-dimer antiferromagnet on the square lattice, for which deviations from O(3) universality have been reported in numerical studies. Using both symmetry arguments and microscopic calculations, we show that a non-trivial cubic term arises in the relevant order-parameter quantum field theory, and assess its consequences using a combination of analytical and numerical methods. We also present finite-temperature quantum Monte Carlo data for the staggered-dimer antiferromagnet which complement recently published results. The data can be consistently interpreted in terms of critical exponents identical to that of the standard O(3) universality class, but with anomalously large corrections to scaling. We argue that the two-particle decay of critical triplons, although irrelevant in two spatial dimensions, is responsible for the leading corrections to scaling due to its small scaling dimension.
Physical Review Letters, 2008
We examine the superfluid and collapse instabilities of a quasi two-dimensional gas of dipolar fermions aligned by an orientable external field. It is shown that the interplay between the anisotropy of the dipole-dipole interaction, the geometry of the system, and the p-wave symmetry of the superfluid order parameter means that the effective interaction for pairing can be made very large without the system collapsing. This leads to a broad region in the phase diagram where the system forms a stable superfluid. Analyzing the superfluid transition at finite temperatures, we calculate the Berezinskii-Kosterlitz-Thouless temperature as a function of the dipole angle. PACS numbers: 03.75.Ss,03.75.Hh Trapped ultracold gases are increasingly being used to simulate solid-state systems, where clear experimental signatures of theoretical predictions are often lacking [1].
Physical Review Letters, 2011
We have studied the transition from two to three dimensions in a low temperature weakly interacting 6 Li Fermi gas. Below a critical atom number, N2D, only the lowest transverse vibrational state of a highly anisotropic oblate trapping potential is occupied and the gas is two-dimensional. Above N2D the Fermi gas enters the quasi-2D regime where shell structure associated with the filling of individual transverse oscillator states is apparent. This dimensional crossover is demonstrated through measurements of the cloud size and aspect ratio versus atom number.
We study the magnetic field driven Quantum Phase Transition (QPT) in electrostatically gated superconducting LaTiO3/SrTiO3 interfaces. Through finite size scaling analysis, we show that it belongs to the (2+1)D XY model universality class. The system can be described as a disordered array of superconducting islands coupled by a two dimensional electron gas (2DEG). Depending on the 2DEG conductance tuned by the gate voltage, the QPT is single (corresponding to the long range phase coherence in the whole array) or double (one related to local phase coherence, the other one to the array). By retrieving the coherence length critical exponent ν, we show that the QPT can be "clean" or "dirty" according to the Harris criteria, depending on whether the phase coherence length is smaller or larger than the island size. The overall behaviour is well described by a theoretical approach of Spivak et al., in the framework of the fermionic scenario of 2D superconducting QPT. interest . Indeed, they display very high mobilities suitable for applications , but also a rich phase diagram, with different quantum ground states such as magnetism or superconductivity[9, 10] for example. Moreover, these properties can be finely tuned using a gate voltage . Therefore, O-2DEG appear as interesting systems to study Quantum Phases Transitions (QPT) that occur between different quantum states, when a parameter in the Hamiltonian crosses over a critical value . The critical behaviour of the observables belong to universality classes which depend on general properties of the system such as its dimensionality or its symmetries, and not on the microscopic details. The associated critical exponents obey specific rules, among which the so-called "Harris criteria". The latter stipulates that the correlation length exponent ν must satisfy ν ≥ 2/d for "dirty" disordered systems and ν ≤ 2/d for "clean" ones, where d is the spatial dimensionality[14]. An important example of QPT is the transition from a superconducting to an insulating state in two dimensions, which has been a matter of debate for a long time . Numerous experiments with contrasted results have been performed, and a large variety of critical exponents have been found. The nature of the non-superconducting state and the role of the disorder are still unclear. The possibility of observing multiple QPT has been raised recently . Here we show that a perpendicular magnetic field applied on a superconducting O-2DEG drives the system towards a weakly localized metal. We evidence two QPT corresponding to the "dirty" and "clean" limits of the Harris criteria, which can be controlled by the gate voltage. More precisely, we have shown that the QPT in
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