slides-SHG enhancement via Fano resonances

We show that, nonlinear optical processes in a plasmonic metal nanoparticle (MNP) dimer can be controlled by the presence of a molecule or a quantum dot. By choosing the appropriate level spacing for the quantum emitter, one can either suppress or enhance the nonlinear frequency conversion. (i) Suppression occurs simply because transparency induced by Fano resonance does not allow an excitation at the converted frequency. (ii) Enhancement emerges since nonlinear process can be brought to resonance. Path interference effect cancels the nonresonant frequency terms. We demonstrate the underlying physics using a simplified model, and we show that the predictions of the model are in good agreement with the 3-dimensional boundary element method (MNPBEM toolbox) simulations. Here, we consider the second harmonic generation in a MNP dimer as an example to demonstrate the control mechanism. However, the method can be easily generalized to other nonlinear processes emerging on plasmonic reson...

Journal of Optics, 2014

We show that, nonlinear optical processes in a plasmonic metal nanoparticle (MNP) dimer can be controlled by the presence of a molecule or a quantum dot. (i) Frequency conversion can be suppressed if the dimer is coupled to a quantum object which is resonant to the generated frequency. This occurs simply because, EIT does not allow an excitation at the converted frequency frequency. (ii) On the contrary, a similar effect can be used to enhance the frequency conversion. Nonlinear processes can be brought to resonance without tuning the dimer modes. Path interference effect cancels the nonresonant frequency terms. Here, we consider the second harmonic generation (SHG) as an example to demonstrate the control mechanism. However, the method can be easily generalized to other nonlinear processes.

Nano Letters, 2016

We present an electrically driven plasmonic device consisting of a gold nanoparticle trapped in a gap between two electrodes. The tunneling current in the device generates plasmons, which decay radiatively. The emitted spectrum extends up to an energy that depends on the applied voltage. Characterization of the electrical conductance at low temperatures allows us to extract the voltage drop on each tunnel barrier and the corresponding emitted spectrum. In several devices we find a pronounced sharp asymmetrical dip in the spectrum, which we identify as a Fano resonance. Finite-difference time-domain (FDTD) calculations reveal that this resonance is due to interference between the nanoparticle and electrodes dipolar fields, and can be conveniently controlled by the structural parameters.

Journal of Applied Physics, 2021

Nature materials, 2010

2011

The Fano resonance of a single symmetry broken Ag nanodisk under a normal incidence was investigated by using finite-difference time-domain (FDTD) simulations. The asymmetry line shape of the Fano resonance was controlled by modifying the open angle of the nanodisk, and this Fano splitting was demonstrated as the result of the overlap between the broad dipolar and narrow quadrupolar modes, which could be strengthened by enlarging the radius of the nanodisk. A semi-analytical method was developed to calculate the plasmon hybridization, which was used to analyze the sub-process of the quadru Fano resonance. With the good agreement between theoretical calculations and FDTD simulations, the suggested method provides a way to investigate and control the Fano resonance inside a single planar nanostructure, and can be applied to the future high-performance Fano resonance sensors.

Plasmonics: Nanoimaging, Nanofabrication, and Their Applications IV, 2008

The optical extinction spectra of single gold nanorods are investigated using a spatial modulation spectroscopy technique. The experimental results are compared to the computed spectra of nanoellipsoids using the dipolar approximation or a generalization of the Mie theory, focussing on the width of the longitudinal surface plasmon resonance. This is shown to be consistent with that deduced from the theoretical models using different available sets of dielectric constant for bulk gold, without introducing surface broadening effect. Extension of this approach to investigation of the ultrafast nonlinear optical response of a single gold nanorod is also discussed.

Springer Theses, 2018

Arxiv preprint physics/ …, 2005

ACS Nano, 2013

Fano resonances in hybridized systems formed from the interaction of bright modes only are reported. Despite precedent works, we demonstrate theoretically and experimentally that Fano resonances can be obtained by destructive interference between two bright dipolar modes out of phase. A simple oscillator model is provided to predict and fit the far-field scattering. The predictions are verified with numerical calculations using a surface integral equation method for a wide range of geometrical parameters. The validity of the model is then further demonstrated with experimental dark-field scattering measurements on actual nanostructures in the visible range. A remarkable set of properties like crossings, avoided crossings, inversion of subradiant and superradiant modes and a plasmonic equivalent of a bound state in the continuum are presented. The nanostructure, that takes advantage of the combination of Fano resonance and nanogap effects, also shows high tunability and strong near-field enhancement. Our study provides a general understanding of Fano resonances as well as a simple tool for engineering their spectral features.