The scientific community is currently very interested in the effect modification of air pollution... more The scientific community is currently very interested in the effect modification of air pollution by meteorological variables. The recent paper by Dr Nawrot and colleagues reports findings from a time-series epidemiology study on the effects of temperature on the association between relative mortality risk and PM10 in Belgium.1 Their 7-year data showed a stronger overall association and no threshold between PM10 and mortality in summer, but a weaker association and a threshold of 30 μg/m3 in winter. Based on these findings they state that “the shape of the dose–response relationship curve between air pollution and mortality strongly depends on outdoor temperature”. We would like to point out that, although a weaker dependency cannot be ruled out, at least a substantial fraction of the observation is most likely attributable to the well-known relationship between personal exposures and air pollution levels at fixed monitoring sites. This relationship is strongly modified by the amount of time spent indoors. Infiltration of outdoor air PM2.5 particles indoors reduces exposure levels relative to ambient levels by 30–40% on average in Europe.2 The associated strong seasonal pattern3 is caused by variation in the times for which windows …
International Journal of Life Cycle Assessment, Nov 21, 2014
Users may download and print one copy of any publication from the public portal for the purpose... more Users may download and print one copy of any publication from the public portal for the purpose of private study or research. You may not further distribute the material or use it for any profit-making activity or commercial gain You may freely distribute the URL identifying the publication in the public portal If you believe that this document breaches copyright please contact us providing details, and we will remove access to the work immediately and investigate your claim.
The intake fraction (iF) has been defined as the integrated incremental intake of a pollutant rel... more The intake fraction (iF) has been defined as the integrated incremental intake of a pollutant released from a source category or region summed over all exposed individuals. In this study we evaluated the iFs in the population of Europe for emissions of anthropogenic primary fine particulate matter (PM 2.5) from sources in Europe, with a more detailed analysis of the iF from Finnish sources. Parameters for calculating the iFs include the emission strengths, the predicted atmospheric concentrations, European population data, and the average breathing rate per person. Emissions for the whole of Europe and Finland were based on the inventories of the European Monitoring and Evaluation Programme (EMEP) and the Finnish Regional Emission Scenario (FRES) model, respectively. The atmospheric dispersion of primary PM 2.5 was computed using the regional-scale dispersion model SILAM. The iFs from Finnish sources were also computed separately for six emission source categories. The iFs corresponding to the primary PM 2.5 emissions from the European countries for the whole population of Europe were generally highest for the densely populated Western European countries, second highest for the Eastern and Southern European countries, and lowest for the Northern European and Baltic countries. For the entire European population, the iF values varied from the lowest value of 0.31 per million for emissions from Cyprus, to the highest value of 4.42 per million for emissions from Belgium. These results depend on the regional distribution of the population and the prevailing long-term meteorological conditions. Regarding Finnish primary PM 2.5 emissions, the iF was highest for traffic emissions (0.68 per million) and lowest for major power plant emissions (0.50 per million). The results provide new information that can be used to find the most cost-efficient emission abatement strategies and policies.
The associations of personal carbon monoxide (CO) exposures with ambient air CO concentrations me... more The associations of personal carbon monoxide (CO) exposures with ambient air CO concentrations measured at fixed monitoring sites, were studied among 194 children aged 3-6 yr in four downtown and four suburban day-care centers in Helsinki, Finland. Each child carried a personal CO exposure monitor between 1 and 4 times for a time period of between 20 and 24 h. CO concentrations at two fixed monitoring sites were measured simultaneously. The CO concentrations measured at the fixed monitoring sites were usually lower (mean maximum 8-h concentration: 0.9 and 2.6 mg m À3) than the personal CO exposure concentrations (mean maximum 8-h concentration: 3.3 mg m À3). The fixed site CO concentrations were poor predictors of the personal CO exposure concentrations. However, the correlations between the personal CO exposure and the fixed monitoring site CO concentrations increased (À0.03-À0.12 to 0.13-0.16) with increasing averaging times from 1 to 8 h. Also, the fixed monitoring site CO concentrations explained the mean daily or weekly personal CO exposures of a group of simultaneously measured children better than individual exposure CO concentrations. This study suggests that the short-term CO personal exposure of children cannot be meaningfully assessed using fixed monitoring sites.
Journal of Exposure Science and Environmental Epidemiology, Jun 1, 1999
In-vehicle exposures to different sizes of particles and carbon monoxide (CO) were determined whi... more In-vehicle exposures to different sizes of particles and carbon monoxide (CO) were determined while driving along a standardized route under a variety of traffic conditions in Kuopio, Finland during the 12-month period from January to December 1995. Arithmetic means of in-vehicle exposures during the morning rush hours were 5.7 parts per million (ppm) (geometric mean, GM=3.1 ppm, geometric standard deviation, GSD=1.7) for CO, 107 #/cm 3 (GM=75 #/ cm 3 , GSD=1.9) for fine particles (optical equivalent particle size range 0.3±1 m) and 0.9 #/cm 3 (GM=0.6 #/cm 3 , GSD=2.1) for coarse particles (optical equivalent particle size range 1±10 m). Fine particles and CO behaved similarly in different weather and traffic conditions, while the behavior of coarse particles was usually different, and often opposite. The driving conditions that affected the passengers' exposures to CO and fine particles were the time of day (morning vs. afternoon) and average speed (decreasing). The meteorological parameters that affected the passengers' exposures to CO and fine particles were wind speed (decreasing) and relative humidity (increasing). Wind speed, relative humidity and driving speed all had opposite effects on the exposure levels to fine vs. coarse particles. Added exposures (due to commuting on top of the background levels) to CO and fine particles were considerably higher in the morning vs. the afternoon runs and also higher in the slower vs. the faster runs.
The European INDEX project was finalised to identify priorities and to assess the needs for an Eu... more The European INDEX project was finalised to identify priorities and to assess the needs for an European Community strategy and action plan in the area of indoor air pollution. A list of 5 chemicals, with potential of high indoor concentrations, uncontested health impacts, and effective risk management, were selected to be regulated with priority: Formaldehyde, Carbon Monoxide, Nitrogen Dioxide, Benzene and Naphtalene. For each compound, guideline values and management options were suggested.JRC.I.5-Physical and chemical exposure
The Practice of Consumer Exposure Assessment, 2019
Users may download and print one copy of any publication from the public portal for the purpose... more Users may download and print one copy of any publication from the public portal for the purpose of private study or research. You may not further distribute the material or use it for any profit-making activity or commercial gain You may freely distribute the URL identifying the publication in the public portal If you believe that this document breaches copyright please contact us providing details, and we will remove access to the work immediately and investigate your claim.
BACKGROUND: The Life Cycle Initiative, hosted at the United Nations Environment Programme, select... more BACKGROUND: The Life Cycle Initiative, hosted at the United Nations Environment Programme, selected human toxicity impacts from exposure to chemical substances as an impact category that requires global guidance to overcome current assessment challenges. The initiative leadership established the Human Toxicity Task Force to develop guidance on assessing human exposure and toxicity impacts. Based on input gathered at three workshops addressing the main current scientific challenges and questions, the task force built a roadmap for advancing human toxicity characterization, primarily for use in life cycle impact assessment (LCIA). OBJECTIVES: The present paper aims at reporting on the outcomes of the task force workshops along with interpretation of how these outcomes will impact the practice and reliability of toxicity characterization. The task force thereby focuses on two major issues that emerged from the workshops, namely considering near-field exposures and improving dose-response modeling. DISCUSSION: The task force recommended approaches to improve the assessment of human exposure, including capturing missing exposure settings and human receptor pathways by coupling additional fate and exposure processes in consumer and occupational environments (near field) with existing processes in outdoor environments (far field). To quantify overall aggregate exposure, the task force suggested that environments be coupled using a consistent set of quantified chemical mass fractions transferred among environmental compartments. With respect to dose-response, the task force was concerned about the way LCIA currently characterizes human toxicity effects, and discussed several potential solutions. A specific concern is the use of a (linear) dose-response extrapolation to zero. Another concern addresses the challenge of identifying a metric for human toxicity impacts that is aligned with the spatiotemporal resolution of present LCIA methodology, yet is adequate to indicate health impact potential. CONCLUSIONS: Further research efforts are required based on our proposed set of recommendations for improving the characterization of human exposure and toxicity impacts in LCIA and other comparative assessment frameworks.
This review set out to identify data sets for airborne chemical pollutants measured in domestic d... more This review set out to identify data sets for airborne chemical pollutants measured in domestic dwellings within European Union (EU) countries from the literature published during 1995–2010. A total of 74 papers satisfied inclusion criteria, and from those papers data on country location, population sampled, sampling period, number of samples and summary statistics of concentrations measured were gathered. The chemical substances identified and included were grouped to aldehydes, radon, carbon dioxide (CO2), carbon monoxide (CO), nicotine, nitrogen dioxide (NO2), polycyclic aromatic hydrocarbons, volatile organic compounds and brominated flame retardants. The review showed that the availability of data between the EU countries is varying and more measured data are available for countries in northern Europe than in the southern parts. This review is part of the Integrated Exposure for Risk Assessment in Indoor Environments project which developed a full-chain modelling platform, inco...
The scientific community is currently very interested in the effect modification of air pollution... more The scientific community is currently very interested in the effect modification of air pollution by meteorological variables. The recent paper by Dr Nawrot and colleagues reports findings from a time-series epidemiology study on the effects of temperature on the association between relative mortality risk and PM10 in Belgium.1 Their 7-year data showed a stronger overall association and no threshold between PM10 and mortality in summer, but a weaker association and a threshold of 30 μg/m3 in winter. Based on these findings they state that “the shape of the dose–response relationship curve between air pollution and mortality strongly depends on outdoor temperature”. We would like to point out that, although a weaker dependency cannot be ruled out, at least a substantial fraction of the observation is most likely attributable to the well-known relationship between personal exposures and air pollution levels at fixed monitoring sites. This relationship is strongly modified by the amount of time spent indoors. Infiltration of outdoor air PM2.5 particles indoors reduces exposure levels relative to ambient levels by 30–40% on average in Europe.2 The associated strong seasonal pattern3 is caused by variation in the times for which windows …
International Journal of Life Cycle Assessment, Nov 21, 2014
Users may download and print one copy of any publication from the public portal for the purpose... more Users may download and print one copy of any publication from the public portal for the purpose of private study or research. You may not further distribute the material or use it for any profit-making activity or commercial gain You may freely distribute the URL identifying the publication in the public portal If you believe that this document breaches copyright please contact us providing details, and we will remove access to the work immediately and investigate your claim.
The intake fraction (iF) has been defined as the integrated incremental intake of a pollutant rel... more The intake fraction (iF) has been defined as the integrated incremental intake of a pollutant released from a source category or region summed over all exposed individuals. In this study we evaluated the iFs in the population of Europe for emissions of anthropogenic primary fine particulate matter (PM 2.5) from sources in Europe, with a more detailed analysis of the iF from Finnish sources. Parameters for calculating the iFs include the emission strengths, the predicted atmospheric concentrations, European population data, and the average breathing rate per person. Emissions for the whole of Europe and Finland were based on the inventories of the European Monitoring and Evaluation Programme (EMEP) and the Finnish Regional Emission Scenario (FRES) model, respectively. The atmospheric dispersion of primary PM 2.5 was computed using the regional-scale dispersion model SILAM. The iFs from Finnish sources were also computed separately for six emission source categories. The iFs corresponding to the primary PM 2.5 emissions from the European countries for the whole population of Europe were generally highest for the densely populated Western European countries, second highest for the Eastern and Southern European countries, and lowest for the Northern European and Baltic countries. For the entire European population, the iF values varied from the lowest value of 0.31 per million for emissions from Cyprus, to the highest value of 4.42 per million for emissions from Belgium. These results depend on the regional distribution of the population and the prevailing long-term meteorological conditions. Regarding Finnish primary PM 2.5 emissions, the iF was highest for traffic emissions (0.68 per million) and lowest for major power plant emissions (0.50 per million). The results provide new information that can be used to find the most cost-efficient emission abatement strategies and policies.
The associations of personal carbon monoxide (CO) exposures with ambient air CO concentrations me... more The associations of personal carbon monoxide (CO) exposures with ambient air CO concentrations measured at fixed monitoring sites, were studied among 194 children aged 3-6 yr in four downtown and four suburban day-care centers in Helsinki, Finland. Each child carried a personal CO exposure monitor between 1 and 4 times for a time period of between 20 and 24 h. CO concentrations at two fixed monitoring sites were measured simultaneously. The CO concentrations measured at the fixed monitoring sites were usually lower (mean maximum 8-h concentration: 0.9 and 2.6 mg m À3) than the personal CO exposure concentrations (mean maximum 8-h concentration: 3.3 mg m À3). The fixed site CO concentrations were poor predictors of the personal CO exposure concentrations. However, the correlations between the personal CO exposure and the fixed monitoring site CO concentrations increased (À0.03-À0.12 to 0.13-0.16) with increasing averaging times from 1 to 8 h. Also, the fixed monitoring site CO concentrations explained the mean daily or weekly personal CO exposures of a group of simultaneously measured children better than individual exposure CO concentrations. This study suggests that the short-term CO personal exposure of children cannot be meaningfully assessed using fixed monitoring sites.
Journal of Exposure Science and Environmental Epidemiology, Jun 1, 1999
In-vehicle exposures to different sizes of particles and carbon monoxide (CO) were determined whi... more In-vehicle exposures to different sizes of particles and carbon monoxide (CO) were determined while driving along a standardized route under a variety of traffic conditions in Kuopio, Finland during the 12-month period from January to December 1995. Arithmetic means of in-vehicle exposures during the morning rush hours were 5.7 parts per million (ppm) (geometric mean, GM=3.1 ppm, geometric standard deviation, GSD=1.7) for CO, 107 #/cm 3 (GM=75 #/ cm 3 , GSD=1.9) for fine particles (optical equivalent particle size range 0.3±1 m) and 0.9 #/cm 3 (GM=0.6 #/cm 3 , GSD=2.1) for coarse particles (optical equivalent particle size range 1±10 m). Fine particles and CO behaved similarly in different weather and traffic conditions, while the behavior of coarse particles was usually different, and often opposite. The driving conditions that affected the passengers' exposures to CO and fine particles were the time of day (morning vs. afternoon) and average speed (decreasing). The meteorological parameters that affected the passengers' exposures to CO and fine particles were wind speed (decreasing) and relative humidity (increasing). Wind speed, relative humidity and driving speed all had opposite effects on the exposure levels to fine vs. coarse particles. Added exposures (due to commuting on top of the background levels) to CO and fine particles were considerably higher in the morning vs. the afternoon runs and also higher in the slower vs. the faster runs.
The European INDEX project was finalised to identify priorities and to assess the needs for an Eu... more The European INDEX project was finalised to identify priorities and to assess the needs for an European Community strategy and action plan in the area of indoor air pollution. A list of 5 chemicals, with potential of high indoor concentrations, uncontested health impacts, and effective risk management, were selected to be regulated with priority: Formaldehyde, Carbon Monoxide, Nitrogen Dioxide, Benzene and Naphtalene. For each compound, guideline values and management options were suggested.JRC.I.5-Physical and chemical exposure
The Practice of Consumer Exposure Assessment, 2019
Users may download and print one copy of any publication from the public portal for the purpose... more Users may download and print one copy of any publication from the public portal for the purpose of private study or research. You may not further distribute the material or use it for any profit-making activity or commercial gain You may freely distribute the URL identifying the publication in the public portal If you believe that this document breaches copyright please contact us providing details, and we will remove access to the work immediately and investigate your claim.
BACKGROUND: The Life Cycle Initiative, hosted at the United Nations Environment Programme, select... more BACKGROUND: The Life Cycle Initiative, hosted at the United Nations Environment Programme, selected human toxicity impacts from exposure to chemical substances as an impact category that requires global guidance to overcome current assessment challenges. The initiative leadership established the Human Toxicity Task Force to develop guidance on assessing human exposure and toxicity impacts. Based on input gathered at three workshops addressing the main current scientific challenges and questions, the task force built a roadmap for advancing human toxicity characterization, primarily for use in life cycle impact assessment (LCIA). OBJECTIVES: The present paper aims at reporting on the outcomes of the task force workshops along with interpretation of how these outcomes will impact the practice and reliability of toxicity characterization. The task force thereby focuses on two major issues that emerged from the workshops, namely considering near-field exposures and improving dose-response modeling. DISCUSSION: The task force recommended approaches to improve the assessment of human exposure, including capturing missing exposure settings and human receptor pathways by coupling additional fate and exposure processes in consumer and occupational environments (near field) with existing processes in outdoor environments (far field). To quantify overall aggregate exposure, the task force suggested that environments be coupled using a consistent set of quantified chemical mass fractions transferred among environmental compartments. With respect to dose-response, the task force was concerned about the way LCIA currently characterizes human toxicity effects, and discussed several potential solutions. A specific concern is the use of a (linear) dose-response extrapolation to zero. Another concern addresses the challenge of identifying a metric for human toxicity impacts that is aligned with the spatiotemporal resolution of present LCIA methodology, yet is adequate to indicate health impact potential. CONCLUSIONS: Further research efforts are required based on our proposed set of recommendations for improving the characterization of human exposure and toxicity impacts in LCIA and other comparative assessment frameworks.
This review set out to identify data sets for airborne chemical pollutants measured in domestic d... more This review set out to identify data sets for airborne chemical pollutants measured in domestic dwellings within European Union (EU) countries from the literature published during 1995–2010. A total of 74 papers satisfied inclusion criteria, and from those papers data on country location, population sampled, sampling period, number of samples and summary statistics of concentrations measured were gathered. The chemical substances identified and included were grouped to aldehydes, radon, carbon dioxide (CO2), carbon monoxide (CO), nicotine, nitrogen dioxide (NO2), polycyclic aromatic hydrocarbons, volatile organic compounds and brominated flame retardants. The review showed that the availability of data between the EU countries is varying and more measured data are available for countries in northern Europe than in the southern parts. This review is part of the Integrated Exposure for Risk Assessment in Indoor Environments project which developed a full-chain modelling platform, inco...
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