Influence of 7Li enrichment on Th-U fuel breeding performance for molten salt reactors under different neutron spectra
Progress in Nuclear Energy, 2020
Abstract To obtain an outstanding neutron economy and Th-U (Thorium-Uranium) breeding performance... more Abstract To obtain an outstanding neutron economy and Th-U (Thorium-Uranium) breeding performance, a quite high 7Li enrichment up to 99.995% is generally required for the designs of molten salt reactors with FLiBe carrier salt. While such high 7Li enrichment would undoubtedly bring great technical challenges and high costs to the molten salt preparation. Meanwhile, the 6Li neutron absorption cross section differs greatly under different neutron spectra, which would probably mean the choice of 7Li enrichment can be different for the molten salt reactors with different neutron spectra. With the aim to provide an appropriate reference for the choice of 7Li enrichment in the engineering design of molten salt reactors, key parameters (including 233U inventory, neutron spectrum, temperature coefficient, 7Li enrichment, 7Li and 6Li neutron absorption rate, breeding ratio, relative 233U production and doubling time) and their time evolution are systematically explored based on the in-house developed code MSR-RS. The results show that 99.99% and 99.95% in 7Li enrichment introduce limited influence on Th-U breeding performance for a thermal and fast reactor respectively, and their temperature coefficient are negative. By trading off the cost and technologies required for enriching 7Li, the above two 7Li enrichment are therefore recommended.
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