Papers by Zbigniew Klimont
Atmospheric Environment, 2009
future changes. Reported results include new estimates of radiative forcing based on extensive mo... more future changes. Reported results include new estimates of radiative forcing based on extensive model studies of chemically active climate compounds like O 3 , and of particles inducing both direct and indirect effects. Through EU projects like ACCENT, QUANTIFY, and the AeroCom project, extensive studies on regional and sector-wise differences in the impact on atmospheric distribution are performed. Studies have shown that land-based emissions have a different effect on climate than ship and aircraft emissions, and different measures are needed to reduce the climate impact. Several areas where climate change can affect the tropospheric oxidation process and the chemical composition are identified. This can take place through enhanced stratospheric-tropospheric exchange of ozone, more frequent periods with stable conditions favoring pollution build up over industrial areas, enhanced temperature induced biogenic emissions, methane releases from permafrost thawing, and enhanced concentration through reduced biospheric uptake. During the last 5-10 years, new observational data have been made available and used for model validation and the study of atmospheric processes. Although there are significant uncertainties in the modeling of composition changes, access to new observational data has improved modeling capability. Emission scenarios for the coming decades have a large uncertainty range, in particular with respect to regional trends, leading to a significant uncertainty range in estimated regional composition changes and climate impact.
Energy Policy, 2001
This paper compares three scenarios of energy demand in the European Union until 2010 and analyse... more This paper compares three scenarios of energy demand in the European Union until 2010 and analyses their effects on carbon emissions as well as their impacts on the precursor emissions for acidification and ground-level ozone. The analysis links the results of energy model PRIMES with the integrated environmental assessment model RAINS. Important synergies between climate change policies and policies to control regional air pollution have been identified. Mitigation of acidification and ozone according to the current EU strategy will be easier and cheaper if the Kyoto targets for the reduction of the emissions of greenhouse gases (GHG) are to be met. In case when the Kyoto target needs to be achieved by individual EU member countries without trading in CO 2 emission rights, the costs of controlling the pollutants contributing to acidification and ground-level ozone can be up to 10% lower than for the baseline scenario which does not assume any climate change policies. Although lower, the effects are also important if trading in carbon emission rights is allowed. These cost savings compensate up to 20% of higher costs of energy supplies in the EU and associated with them welfare losses caused by the necessity to meet the carbon constraint. #
Science, 2012
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Environmental health perspectives, 2012
Tropospheric ozone and black carbon (BC), a component of fine particulate matter (PM ≤ 2.5 µm in ... more Tropospheric ozone and black carbon (BC), a component of fine particulate matter (PM ≤ 2.5 µm in aerodynamic diameter; PM(2.5)), are associated with premature mortality and they disrupt global and regional climate. We examined the air quality and health benefits of 14 specific emission control measures targeting BC and methane, an ozone precursor, that were selected because of their potential to reduce the rate of climate change over the next 20-40 years. We simulated the impacts of mitigation measures on outdoor concentrations of PM(2.5) and ozone using two composition-climate models, and calculated associated changes in premature PM(2.5)- and ozone-related deaths using epidemiologically derived concentration-response functions. We estimated that, for PM(2.5) and ozone, respectively, fully implementing these measures could reduce global population-weighted average surface concentrations by 23-34% and 7-17% and avoid 0.6-4.4 and 0.04-0.52 million annual premature deaths globally in ...
We evaluate black carbon (BC) model predictions from the AeroCom model intercomparison project by... more We evaluate black carbon (BC) model predictions from the AeroCom model intercomparison project by considering the diversity among year 2000 model simulations and comparing model predictions with available measurements. These model-measurement intercomparisons include BC surface and aircraft concentrations, aerosol absorption optical depth (AAOD) retrievals from AERONET and Ozone Monitoring Instrument (OMI) and BC column estimations based on AERONET. In regions other than Asia, most models are biased high compared to surface concentration measurements. However compared with (column) AAOD or BC burden retreivals, the models are generally biased low. The average ratio of model to retrieved AAOD is less than 0.7 in South American and 0.6 in African biomass burning regions; both of these regions lack surface concentration measurements. In Asia the average model to observed ratio is 0.7 for AAOD and 0.5 for BC surface concentrations. Compared with aircraft measurements over the Americas at latitudes between 0 and 50N, the average model is a factor of 8 larger than observed, and most models exceed the measured BC standard deviation in the mid to upper troposphere. At higher latitudes the average model to aircraft BC ratio is 0.4 and models underestimate the observed BC loading in the lower and middle troposphere associated with springtime Arctic haze. Low model bias for AAOD but overestimation of surface and upper atmospheric BC concentrations at lower latitudes suggests that most models are underestimating BC absorption and should improve estimates for refractive index, particle size, and optical effects of BC coating. Retrieval uncertainties and/or differences with model diagnostic treatment may also contribute to the model-measurement disparity. Largest AeroCom model diversity occurred in northern Eurasia and the remote Arctic, regions influenced by anthropogenic sources. Changing emissions, aging, removal, or optical properties within a single model generated a smaller change in model predictions than the range represented by the full set of AeroCom models. Upper tropospheric concentrations of BC mass from the aircraft measurements are suggested to provide a unique new benchmark to test scavenging and vertical dispersion of BC in global models.
The 2007 IPCC Fourth Assessment Report noted that black carbon (BC) may exert a significant anthr... more The 2007 IPCC Fourth Assessment Report noted that black carbon (BC) may exert a significant anthropogenic warming effect on the global climate. Since then an increasing number of modeling and sampling studies have strongly supported this warming effect. This is especially true in the Arctic and other snow-covered regions, where BC in the atmosphere absorbs more heat over these reflective surfaces; and once deposited, darkens snow and ice to lead to greater melting as well. The melting leads to greater exposure of the darker land and sea below, which in turn absorb more heat, and thus to additional warming and melting.
The 2007 IPCC Fourth Assessment Report noted that black carbon (BC) may exert a significant anthr... more The 2007 IPCC Fourth Assessment Report noted that black carbon (BC) may exert a significant anthropogenic warming effect on the global climate. Since then an increasing number of modeling and sampling studies have strongly supported this warming effect. This is especially true in the Arctic and other snow-covered regions, where BC in the atmosphere absorbs more heat over these reflective surfaces; and once deposited, darkens snow and ice to lead to greater melting as well. The melting leads to greater exposure of the darker land and sea below, which in turn absorb more heat, and thus to additional warming and melting.
Atmospheric Chemistry and Physics, 2015
ABSTRACT The global aerosol--climate model ECHAM-HAMMOZ is used to study the aerosol burden and f... more ABSTRACT The global aerosol--climate model ECHAM-HAMMOZ is used to study the aerosol burden and forcing changes in the coming decades. We show that aerosol burdens overall can have a decreasing trend leading to reductions in the direct aerosol effect being globally 0.06--0.4W/m2 by 2030, whereas the aerosol indirect radiative effect could decline 0.25--0.82W/m2. We also show that the targeted emission reduction measures can be a much better choice for the climate than overall high reductions globally.
International Institute for Applied Systems Analysis Schlossplatz 1 A-2361 Laxenburg Austria ... more International Institute for Applied Systems Analysis Schlossplatz 1 A-2361 Laxenburg Austria Telephone: (+43 2236) 807 Fax: (+43 2236) 807 533 E-mail: [email protected] Internet: www.iiasa.ac.at ... The Convention on Long-range Transboundary Air Pollution ...
Energy Strategy Reviews, 2012
Atmospheric Chemistry and Physics Discussions, 2014
ABSTRACT Ozone and PM2.5 concentrations over the city of Paris are modeled with the CHIMERE air-q... more ABSTRACT Ozone and PM2.5 concentrations over the city of Paris are modeled with the CHIMERE air-quality model at 4 km × 4 km horizontal resolution for two future emission scenarios. High-resolution (1 km × 1 km) emission projection until 2020 for the greater Paris region is developed by local experts (AIRPARIF) and is further extended to year 2050 based on regional scale emission projections developed by the Global Energy Assessment. Model evaluation is performed based on a 10 yr control simulation. Ozone is in very good agreement with measurements while PM2.5 is underestimated by 20% over the urban area mainly due to a large wet bias in wintertime precipitation. A significant increase of maximum ozone relative to present time levels over Paris is modeled under the "business as usual" scenario (+7 ppb) while a more optimistic mitigation scenario leads to moderate ozone decrease (-3.5 ppb) in year 2050. These results are substantially different to previous regional scale projections where 2050 ozone is found to decrease under both future scenarios. A sensitivity analysis showed that this difference is due to the fact that ozone formation over Paris at the current, urban scale study, is driven by VOC-limited chemistry, whereas at the regional scale ozone formation occurs under NOx-sensitive conditions. This explains why the sharp NOx reductions implemented in the future scenarios have a different effect on ozone projections at different scales. In rural areas projections at both scales yield similar results showing that the longer time-scale processes of emission transport and ozone formation are less sensitive to model resolution. PM2.5 concentrations decrease by 78% and 89% under "business as usual" and "mitigation" scenarios respectively compared to present time period. The reduction is much more prominent over the urban part of the domain due to the effective reductions of road transport and residential emissions resulting in the smoothing of the large urban increment modelled in the control simulation.
Science of The Total Environment, 2015
Ozone and PM2.5 are current risk factors for premature death all over the globe. In coming decade... more Ozone and PM2.5 are current risk factors for premature death all over the globe. In coming decades, substantial improvements in public health may be achieved by reducing air pollution. To better understand the potential of emissions policies, studies are needed that assess possible future health impacts under alternative assumptions about future emissions and climate across multiple spatial scales. We used consistent climate-air-quality-health modeling framework across three geographical scales (World, Europe and Ile-de-France) to assess future (2030-2050) health impacts of ozone and PM2.5 under two emissions scenarios (Current Legislation Emissions, CLE, and Maximum Feasible Reductions, MFR). Consistently across the scales, we found more reductions in deaths under MFR scenario compared to CLE. 1.5 [95% CI: 0.4, 2.4] million CV deaths could be delayed each year in 2030 compared to 2010 under MFR scenario, 84% of which would occur in Asia, especially in China. In Europe, the benefits under MFR scenario (219000 CV deaths) are noticeably larger than those under CLE (109000 CV deaths). In Ile-de-France, under MFR more than 2830 annual CV deaths associated with PM2.5 changes could be delayed in 2050 compared to 2010. In Paris, ozone-related respiratory mortality should increase under both scenarios. Multi-scale HIAs can illustrate the difference in direct consequences of costly mitigation policies and provide results that may help decision-makers choose between different policy alternatives at different scales.
Atmospheric Environment, 2014
ABSTRACT Diesel vehicles are a significant source of black carbon (BC) and ozone precursors, whic... more ABSTRACT Diesel vehicles are a significant source of black carbon (BC) and ozone precursors, which are important contributors to climate warming, degrade air quality and harm human health. Reducing diesel emissions could mitigate near-term climate change with significant co-benefits. This study quantifies the global and regional climate impacts of BC and co-emitted short-lived climate forcers (SLCFs) from present-day on-road diesel vehicles, as well as future impacts following a current legislation emission scenario. Atmospheric concentrations are calculated by the chemical transport model OsloCTM2. The following radiative forcing (RF) and equilibrium surface temperature responses are estimated. For year 2010 on-road diesel emissions we estimate a global-mean direct RF from BC of 44 m W/m2 and an equilibrium surface temperature response of 59 mK, including the impact of BC deposition on snow. Accounting for cooling and warming impacts of co-emitted SLCFs results in a net global-mean RF and warming of 28 mW/m2 and 48 mK, respectively. Using the concept of Regional Temperature change Potential (RTP), we find significant geographical differences in the responses to regional emissions. Accounting for the vertical sensitivities of the forcing/response relation amplifies these differences. In terms of individual source regions, emissions in Europe give the largest regional contribution to equilibrium warming caused by year 2010 on-road diesel BC, while Russia is most important for Arctic warming per unit emission. The largest contribution to warming caused by the year 2050 on-road diesel sector is from emissions in South Asia, followed by East Asia and the Middle East. Hence, in regions where current legislation is not sufficient to outweigh the expected growth in activity, accelerated policy implementation is important for further future mitigation.
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Papers by Zbigniew Klimont